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It has been suggested that the psychostimulant effects of caffeine depend on its ability to block an allosteric modulation within the A2AR-D2R heteromer, by which adenosine decreases the affinity and intrinsic efficacy of dopamine at the D2R.
"The effect of caffeine on intraocular pressure: a systematic review and meta-analysis".
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Unlike many other psychoactive substances, it is legal and unregulated in nearly all parts of the world.
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"Methylxanthines are the psycho-pharmacologically active constituents of chocolate".
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173 "Decaffeinated" coffees do in fact contain caffeine in many cases  some commercially available decaffeinated coffee products contain considerable levels.
Doherty M, Smith PM (April 2005).